Density Accelerated Relaxation in Active Passive Colloidal Networks with Competing Interactions

Overview & Synopsis

We investigate quasi-2D active-passive colloidal mixtures with electric field-mediated non-identical interactions: unlike species attract and like species repel. Mapping the steady states across total area fraction and active particle area fraction identifies the regime of active percolated network formation among active fluid and clustered states. Within the percolated network regime, relaxation speeds up with increasing density, contrary to expectations for dense particulate gels. Particle-resolved dynamics and microstructure link this acceleration to activity-driven rearrangements enabled by asymmetric interactions.